Synthesis of Xanthones via Copper(II)-Catalyzed Dehydrogenative Cyclization and Successive Aromatization in a One-Step Sequence

  • Jang, Yoon Hu
  • Yang, Yo-Sep
  • Son, Seung Hwan
  • Yoo, Hyung-Seok
  • Shin, Jeong-Won
  • 외 4명
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초록

In this study, an unprecedented approach to the xanthone scaffold from cyclohexyl(2-hydroxyphenyl)methanone via dehydrogenative cyclization and a successive aromatization cascade is reported. This methodology affords a novel route to the privileged structure with a wide substrate scope (a total of 29 compounds, <= 96% yield) in a highly atom-economic manner.

키워드

PHENOLSOXYGEN
제목
Synthesis of Xanthones via Copper(II)-Catalyzed Dehydrogenative Cyclization and Successive Aromatization in a One-Step Sequence
저자
Jang, Yoon HuYang, Yo-SepSon, Seung HwanYoo, Hyung-SeokShin, Jeong-WonWon, Hyuck-JaeKim, Soo LimLim, ChangjinKim, Nam-Jung
DOI
10.1021/acs.orglett.2c03730
발행일
2022-12-23
유형
Article
저널명
Organic Letters
24
50
페이지
9216 ~ 9221